University Of Groningen Polarization Transfer In Ion .

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University of GroningenPolarization transfer in ion-surface scatteringWinters, Danyal Ferdinant AlexanderIMPORTANT NOTE: You are advised to consult the publisher's version (publisher's PDF) if you wish to cite fromit. Please check the document version below.Document VersionPublisher's PDF, also known as Version of recordPublication date:2004Link to publication in University of Groningen/UMCG research databaseCitation for published version (APA):Winters, D. F. A. (2004). Polarization transfer in ion-surface scattering Groningen: s.n.CopyrightOther than for strictly personal use, it is not permitted to download or to forward/distribute the text or part of it without the consent of theauthor(s) and/or copyright holder(s), unless the work is under an open content license (like Creative Commons).Take-down policyIf you believe that this document breaches copyright please contact us providing details, and we will remove access to the work immediatelyand investigate your claim.Downloaded from the University of Groningen/UMCG research database (Pure): http://www.rug.nl/research/portal. For technical reasons thenumber of authors shown on this cover page is limited to 10 maximum.Download date: 10-02-2018

Polarization transferinion-surface scattering

Omslag: Photograph of a water reflection. All reflections from objects abovewater are partially polarized.This work is sponsored by the ’Stichting voor Fundamenteel Onderzoek der Materie’ (FOM) which is financially supported by the ’Nederlandse organisatievoor Wetenschappelijk Onderzoek’ (NWO).Druk: Drukkerij Van Denderen, Groningen, april 2004.

RIJKSUNIVERSITEIT GRONINGENPolarization transferinion-surface scatteringProefschriftter verkrijging van het doctoraat in deWiskunde en Natuurwetenschappenaan de Rijksuniversiteit Groningenop gezag van deRector Magnificus, dr. F. Zwarts,in het openbaar te verdedigen opvrijdag 7 mei 2004 om16.15 uurdoorDanyal Ferdinant Alexander Wintersgeboren op 25 maart 1973te Meppel

Promotores:Prof. dr. R. MorgensternProf. dr. ir. R. HoekstraBeoordelingscommissie:Prof. dr. W. HeilandProf. dr. R.G.E. TimmermansProf. dr. L. Niesen

Contents1 General introduction1.1 Introduction . . . . . .1.2 Ion-surface interaction1.3 Alternative techniques1.4 This thesis . . . . . . .112452 Ion-surface fundamentals2.1 Introduction . . . . . . . . . . .2.2 Classical over the barrier model2.3 Reaction processes . . . . . . .2.3.1 Resonant transitions . .2.3.2 Collective excitations . .2.3.3 Auger neutralization . .2.3.4 Auger de-excitation . .2.3.5 Autoionization . . . . .2.3.6 Radiative decay . . . . .778111113131415163 Experiment3.1 Introduction . . . . . . . . . . .3.2 ECRIS . . . . . . . . . . . . . .3.3 Surface physics setup . . . . . .3.3.1 Beam deceleration . . .3.3.2 Electrostatic analyzer .3.3.3 Photon detection system3.3.4 Polarization analysis . .3.3.5 Sample holders . . . . .1919212225262931334 Sputtering of hollow carbon atoms4.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.2 Sample preparation . . . . . . . . . . . . . . . . . . . . . . . . .4.3 Results . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .35353536.v

CONTENTSvi4.44.5Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .Summary . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .5 Spin-polarized surfaces5.1 Introduction . . . . . . . . . . . . . . . . .5.2 Spin polarization by optical pumping . . .5.3 Temperature dependent spin polarization5.4 Magnetically induced spin polarization . .4047.49494955576 Atomic features of Auger spectra6.1 Introduction . . . . . . . . . . . . . . . . . .6.2 Helium electronic structure . . . . . . . . .6.3 The free atom model . . . . . . . . . . . . .6.4 Auger spectra: metal versus semiconductor6.4.1 Target electronic structure . . . . . .6.4.2 Resonant ionization . . . . . . . . .6.4.3 State population . . . . . . . . . . .6.4.4 Modified DOS . . . . . . . . . . . .6.4.5 Parallel velocity . . . . . . . . . . .6.4.6 Spin ordering . . . . . . . . . . . . .67676869717576798083847 Summary and outlook87Atomic units91KLL Auger energies93Nederlandse samenvatting101Dankwoord105

ion-surface scattering Proefschrift ter verkrijging van het doctoraat in de Wiskunde en Natuurwetenschappen aan de Rijksuniversiteit Groningen op gezag van de Rector Magnificus, dr. F. Zwarts, in het openbaar te verdedigen op vrijdag 7 mei 2004 om 16.15 uur door Danyal Ferdinant Alexander Winters geboren op 25 maart 1973 te Meppel

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